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简介 冷原子物理、非线性物理与光学、自旋电子材料、介观超导、软物质以及生物物理、机器学习等领域

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First-Principles Study of Hole-Doped Superconductors RNiO<sub>2</sub> (R = Nd, La, and Pr)

2022
期刊 Chinese Physics Letters
Recent experiments have found that in contrast to the nonsuperconducting bulk RNiO2 (R = Nd, La, and Pr), the strontium-doped R 1 – x Sr x NiO 2 thin films show superconductivity with the critical temperature T c of 9–15 K at x = 0.2, whose origin of superconductivity deserves further investigation. Based on first-principles calculations, we study the electronic structure, lattice dynamics, and electron–phonon coupling (EPC) of the undoped and doped RNiO2 (R = Nd, La, and Pr) at the experimental doping level. Our results show that the EPC-derived T c’s are all about 0 K in the undoped and doped RNiO2. The electron–phonon coupling strength is too small to account for the observed superconductivity. We hence propose that the electron–phonon interaction can not be the exclusive origin of the superconductivity in RNiO2 (R = Nd, La, and Pr).